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• W2000523661 abstract "The interaction of CO2 with clean Li at 120–320 K was studied using photoelectron spectroscopy. To assist in the interpretation of the spectra, the C 1s and O 1s core-level binding energies of various Li cluster compounds were calculated using an ab initio SCF method. To further understand the reaction pathway, we also studied the reaction of CO2 with an O2 pre-dosed Li surface, and the adsorption of CO on clean Li. The principal reactions occurring between CO2 (1–30 L) and Li at 120–320 K are: CO2⇒[CO2]ads, 2[CO2]ads⇒CO2−3+COads, probably via an oxalate, [C2O4]ads, intermediate, and: COads⇒C+O2−, CO2+O2−⇒CO2−3. The relative rates of these reactions are temperature dependent. At 120 K, the main products are CO2−3, COads, and [CO2]ads, whereas at 320 K the main products are O2− and elemental carbon with a relatively small amount of CO2−3. The reactions are similar to those on the other alkali metals, Na, K and Cs, with the important exception being the much stronger interaction with CO, leading to dissociation and carbon formation." @default.
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• W2000523661 date "1998-11-01" @default.
• W2000523661 modified "2023-10-03" @default.
• W2000523661 title "The reaction of lithium with carbon dioxide studied by photoelectron spectroscopy" @default.
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• W2000523661 doi "https://doi.org/10.1016/s0039-6028(98)00710-9" @default.
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