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- W2000540458 abstract "Recently, time-dependent perturbation theory has been used to investigate single- and multi-photon elliptical and circular dichroism for molecules having permanent electric dipole, and both permanent and transition electric quadrupole, moments in addition to the more commonly treated transition electric and magnetic dipole moments. In this paper it is shown how analytic rotating-wave approximation (RWA) expressions for the transition probabilities for a two-level molecule, having all the relevant transition and permanent moments and interacting with elliptically polarized light, can be employed to augment the perturbative treatments of chiroptical effects. Examples are given which illustrate how the RWA can be used, unlike the perturbative treatments, to study circular dichroism for long times, and for absorption spectra, including effects of permanent multipole moments absent in the perturbative analysis. Some of the effects of permanent moments on the single- and multi-photon circular and elliptical dichroism for chiral molecules are discussed. For example, two-photon dichroism, for molecules with permanent multipole moments, can offer a very different and more detailed probe of molecular structure than the usual one-photon circular dichroism." @default.
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- W2000540458 title "Single- and multi-photon circular and elliptical dichroism — the effects of permanent multipole moments and molecular structure" @default.
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- W2000540458 doi "https://doi.org/10.1016/0166-1280(91)85242-y" @default.
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