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- W2000558232 abstract "The synthesis and solid-state structural characterization of a family of homoleptic and mixed dialkyl d1Ta(IV) complexes of the formula, (η5-C5Me5)TaR1R2[N(i-Pr)C(Me)N(i-Pr)], where R1 = R2 = i-Bu (3), n-Bu (4), and Et (7), and R1 = Me, R2 = i-Bu (10), neopentyl (Np) (11), are reported, along with those for the cationic d1Ta(IV) complex, {(η5-C5Me5)TaNp[N(i-Pr)C(Me)N(i-Pr)]}[B(C6F5)4] (12). All of the new compounds displayed a remarkably high degree of solution stability toward β-hydrogen and β-methyl eliminations/abstractions. Thermolysis of 3 in toluene at 80 °C for 18 h provided the Ta(IV) trimethylenemethane (TMM) complex 13." @default.
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- W2000558232 date "2006-11-21" @default.
- W2000558232 modified "2023-10-14" @default.
- W2000558232 title "High-Oxidation-State Neutral and Cationic Tantalum(IV) Alkyl Complexes That Are Stable toward β-Hydrogen and β-Methyl Eliminations" @default.
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- W2000558232 doi "https://doi.org/10.1021/ja067011y" @default.
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