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• W2000575276 abstract "Surface layers on the French borosilicate nuclear waste glass, R7T7, corroded in MgCl2 solution were studied to determine the composition, structure and stability of crystalline phases. The characteristics of the phases constituting the surface layer varied with the parameter SV × t, the glass surface area (S) to solution volume (V) ratio, times time (t). At low SV × t values (< 360 days/m; ≤ 36 d) th surface layer was thin and contained mainly iron hydroxide particles and hydrotalcite crystals. At an intermediate SV × t value (2800 d/m; 5.5 y) the surface layer contained hydrotalcite-, chlorite- and saponite-type phases. At the highest SV × t value (107 d/m; 463 d) the major phases were saponite, powellite, barite and cerianite solid solutions. About 95% of the uranium and > 98% of the neodymium released from the glass were precipitated in the surface layer. In the 463 day experiment, 86% of the neodymium in the surface layer was in solid solution with powellite, the rest with saponite. Uranium was contained exclusively in saponite. High SV ratios, typical of disposal conditions for vitrified high-level radioactive waste, favor retention of actinides in fairly insoluble corrosion products. Observation of similar corrosion products on natural glasses as on nuclear waste glasses lend support to the hypothesis that the host phases for actinides observed in the laboratory are stable over geological periods of time." @default.
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• W2000575276 date "1997-01-01" @default.
• W2000575276 modified "2023-09-25" @default.
• W2000575276 title "Surface layers on a borosilicate nuclear waste glass corroded in MgCl2 solution" @default.
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• W2000575276 doi "https://doi.org/10.1016/s0022-3115(96)00672-1" @default.
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