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- W2000581631 abstract "We apply and explore techniques aiming at enhancing the tunneling by laser fields, originally developed for a one-dimensional model, to a complete six-dimensional vibrational model of the inversion motion in NHD(2). The computational study is performed with the multi-configuration time-dependent Hartree method. Assuming an ideal three-dimensional alignment we obtain a driven tunneling time twenty times smaller than the natural one, in rather good agreement with an oversimplified three-state model. In the case of one-dimensional alignment, a linearly polarized field leads to a poor enhancement of the tunneling probability, after averaging over the rotation about the alignment axis, whereas a circularly polarized field improves the rotationally averaged tunneling probability at the end of the pulse." @default.
- W2000581631 created "2016-06-24" @default.
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- W2000581631 date "2012-05-21" @default.
- W2000581631 modified "2023-10-17" @default.
- W2000581631 title "Laser-induced enhancement of tunneling in NHD<sub>2</sub>" @default.
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- W2000581631 doi "https://doi.org/10.1063/1.4718591" @default.
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- W2000581631 hasPublicationYear "2012" @default.
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