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• W2000595055 abstract "We derive the rheologically relevant “priority” and “seniority” distributions of entangled segment topology from a kinetic model of long chain branch formation in metallocene-catalyzed polyolefins. For the model considered, the chemistry results in a two-parameter family of molecular distributions; convenient parameters are the typical strand molecular weight between cross-links and a branching probability. Only the branching probability controls the chain topologies. We comment on the different nature of the metallocene ensemble from the usual gelation ensemble that is a candidate model for standard low-density polyethylene. We calculate the extensional rheology of a model system within a decoupling approximation that permits a partial mapping onto the “multimode pompom” constitutive scheme." @default.
• W2000595055 created "2016-06-24" @default.
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• W2000595055 date "2001-02-14" @default.
• W2000595055 modified "2023-10-17" @default.
• W2000595055 title "Molecular Rheology and Statistics of Long Chain Branched Metallocene-Catalyzed Polyolefins" @default.
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• W2000595055 doi "https://doi.org/10.1021/ma001483u" @default.
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