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- W2000599557 abstract "Dissipative particle dynamics simulations of a mesoscale model are performed to investigate the concentration dependence of surfactant adsorption on small-diameter carbon nanotubes and their bundles. Adsorption is found to follow fundamentally different mechanisms in the two cases because of the heterogeneity of the bundle surface and the difference in diameter of bundles compared to that of individual tubes. Whereas aggregation dominates adsorption on individual tubes, on bundles it is largely a Langmuir-type process. High adsorption energy sites on the outer surface of bundles, where surfactant molecules can interact with two tubes simultaneously, dominate at low coverage. They also cause adsorption on bundles to become significant well before adsorption on individual tubes starts. The difference in the adsorption mechanisms leads to a crossover point at higher concentrations, where the adsorbed amount per surface area on individual tubes becomes larger than that for the bundles." @default.
- W2000599557 created "2016-06-24" @default.
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- W2000599557 date "2009-10-19" @default.
- W2000599557 modified "2023-10-14" @default.
- W2000599557 title "The Differences in Surfactant Adsorption on Carbon Nanotubes and Their Bundles" @default.
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- W2000599557 doi "https://doi.org/10.1021/la902376b" @default.
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