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• W2000604578 abstract "We report on theoretical investigations of the exotic magnetism in rubidium sesquioxide Rb4O6, a model correlated system with an open 2p shell. Experimental investigations indicated that Rb4O6 is a magnetically frustrated insulator. The frustration is explained here by electronic structure calculations that incorporate the correlation between the oxygen 2p electrons and deal with the mixed-valent oxygen. This leads to a physical picture where the symmetry is reduced because one third of the oxygen in Rb4O6 is nonmagnetic while the remaining two thirds assemble in antiferromagnetic arrangements. A degenerate, insulating ground state with a large number of frustrated noncollinear magnetic configurations is confidently deduced from the theoretical point of view. These findings demonstrate in general the importance of electron-electron correlations in open-shell p-electron systems." @default.
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• W2000604578 date "2009-01-05" @default.
• W2000604578 modified "2023-10-02" @default.
• W2000604578 title "Challenge of Magnetism in Strongly Correlated Open-Shell<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mn>2</mml:mn><mml:mi>p</mml:mi></mml:math>Systems" @default.
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• W2000604578 doi "https://doi.org/10.1103/physrevlett.102.016401" @default.
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