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- W2000624097 abstract "Abstract A simple, inelastic electron-scattering dynamical model is presented to account for vibrational excitation in molecular adsorbates. The basic two ingredients of the theoretical model are: (i) the conservation of the total angular momentum, and (ii) the requirement of a critical time to allow for the intra-molecular energy re-arrangement of the transient negative-ion complex. The model is applied to the vibrational excitation dynamics of molecules chemisorbed at sub-monolayer conditions on ordered metal surfaces. This was exemplified for Acrylonitrile adsorbed on Cu(1 0 0), whose vibrational excitation was studied via energy loss spectra of low-energy two-photon photoemission (2PPE) electrons, and for ammonia (NH 3 and ND 3 ) adsorbed on Cu(1 0 0), being probed in a STM experiment. Fits of the model to the data allowed for deducing the energy threshold of the vibrational excitation of the C C and C N bonds of the ACN adsorbate molecules, and the threshold for the symmetric ν 1 -stretch mode excitation of adsorbed NH 3 /ND 3 . Also, information about the temporal dynamics underlying the inelastic electron scattering was gained." @default.
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- W2000624097 date "2013-01-01" @default.
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- W2000624097 title "Vibrational excitation of adsorbed molecules by low-energy photon-emitted electrons: A dynamical model" @default.
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- W2000624097 doi "https://doi.org/10.1016/j.molstruc.2012.07.032" @default.
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