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- W2000636758 abstract "The dismutation of uranium(V) in carbonate-bicarbonate solutions has been studied by means of cyclic chronopotentiometry. The aim of the investigation has been to elucidate the actual reaction mechanism. There is evidence from the data on the concentration and pH dependence of the rate coefficients for the dismutation of uranium(V) that the disproportionation reaction is paralleled by an e.c.e. mechanism. The e.c.e. path contributes significantly to the overall reaction rate for concentrations of free carbonate ion of 5×10−3 M and of U(VI) of 1 and 3×10−3 M. For higher concentrations of either the free carbonate or of U(VI) in the bulk of solution the disproportionation is the predominant mechanism. It is difficult, if not even impossible, with the presently available electrochemical techniques, to estimate the relative contributions of either reaction mechanism." @default.
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- W2000636758 date "1974-07-01" @default.
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- W2000636758 title "An investigation of the dismutation of uranium(V) in sodium bicarbonate-carbonate solutions with cyclic chronopotentiometry" @default.
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- W2000636758 doi "https://doi.org/10.1016/s0022-0728(74)80392-x" @default.
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