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• W2000644583 abstract "The relationship between Wigner crystallization of the classical ionic plasma and the liquid-solid transition of alkali metals is examined within the density wave theory of freezing. Freezing of the classical plasma on a rigid neutralizing background into the BCC structure is first re-evaluated, in view of recent progress in the determination of its thermodynamic functions by simulation. Freezing into the FCC structure is also considered in this context and found to be not favoured. On allowing for long-wavelength deformability of the background, the ensuing appearance of a volume change on freezing into the BCC structure is accompanied by reduced stability of the fluid phase and by an increase in the entropy of melting. Freezing all alkali metals into the BCC structure is next evaluated, taking their ionic pair structure as that of an ionic plasma reference fluid screened by conduction electrons and requiring that the correct ionic coupling strength at liquid-solid coexistence should be approximately reproduced. The ensuing values of the volume and entropy changes across the phase transition are in reasonable agreement with experiment. The order parameters of the phase transition, excepting the (200) one, conform rather closely to Gaussian behaviour and yield a Lindemann ratio in reasonable agreement with the empirical value for melting of BCC crystals." @default.
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• W2000644583 date "1991-03-18" @default.
• W2000644583 modified "2023-09-25" @default.
• W2000644583 title "Freezing of liquid alkali metals as screened ionic plasmas" @default.
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• W2000644583 doi "https://doi.org/10.1088/0953-8984/3/11/020" @default.
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