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• W2000647330 abstract "Through-ligand electronic coupling in the [(NH3)5RuIII—1,4-dicyanobenzene—RuII(NH3)5]5+ complex is calculated depending on the donor or acceptor grafted on the benzene. The coupling strength is first discussed, showing that through-dicyanobutadiene is larger than through-1,4-dicyanobenzene coupling. With this ligand, the largest electronic coupling is reached with a full 4NO2 substitution on the benzene. Coupling through an asymmetric 2NO22NH2-substituted benzene is one order of magnitude lower. This large difference is interpreted using the number and position of the active ligand molecular orbitals relative to the d-ruthenium orbital." @default.
• W2000647330 created "2016-06-24" @default.
• W2000647330 creator A5088421071 @default.
• W2000647330 date "1991-10-01" @default.
• W2000647330 modified "2023-09-25" @default.
• W2000647330 title "Tuning of through-bond electronic coupling by donor and acceptor substitutions in the [(NH3)5Ru—1,4-dicyanobenzene—Ru(NH3)5]5+ complex" @default.
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• W2000647330 doi "https://doi.org/10.1016/0009-2614(91)80261-u" @default.
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