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- W2000647392 abstract "We present a theoretical investigation of the effect of spin manipulation of polaron pairs (PPs) on the conductivity of organic semiconductors. Control of the PP spin state is achieved using pulsed electron-spin resonance. We demonstrate that manipulation of PPs will result in changes in the free-polaron density in the material, with corresponding changes in the conductivity due to the contribution of PP dissociation to the free-carrier density. The time-dependent form of this conductivity change following spin resonant perturbation is determined, and the effect of a number of experimental variables investigated. We find that, under certain conditions, these time-dependent current measurements reveal the dynamics of PP intersystem crossing. We compare these predictions with previous experiments on organic light-emitting diodes made of poly[2-methoxy-5-(${2}^{ensuremath{'}}$-ethyl-hexyloxy)-1,4-phenylene vinylene] and conclude that PP intersystem crossing times ${ensuremath{tau}}_{isc}$ in this material may exceed $10text{ }ensuremath{mu}text{s}$ at low temperatures." @default.
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- W2000647392 date "2010-09-13" @default.
- W2000647392 modified "2023-09-26" @default.
- W2000647392 title "Spin-dependent dynamics of polaron pairs in organic semiconductors" @default.
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- W2000647392 doi "https://doi.org/10.1103/physrevb.82.125206" @default.
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