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- W2000648605 abstract "We investigate the incoherent diffusion of excitons in thin films ($5.1ifmmodepmelsetextpmfi{}0.1text{ }text{nm}$ thick) of a highly absorbing J-aggregated cyanine dye material (${10}^{6}text{ }{text{cm}}^{ensuremath{-}1}$ absorption constant) as the excitonic component of a polariton microcavity. Under high-intensity pulsed laser excitation, the J-aggregated molecular films exhibit significant exciton-exciton annihilation, indicating a large exciton diffusion radius of more than 100 nm. When the material is strongly coupled to a cavity, the polaritonic structure also shows exciton-exciton annihilation, which is a competing process against the establishment of a threshold population of polaritons needed for polariton lasing. This study suggests that exciton-exciton annihilation is a loss process which can significantly increase the lasing threshold in polariton microcavities." @default.
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- W2000648605 date "2010-09-27" @default.
- W2000648605 modified "2023-10-18" @default.
- W2000648605 title "Exciton-exciton annihilation in organic polariton microcavities" @default.
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- W2000648605 doi "https://doi.org/10.1103/physrevb.82.113106" @default.
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