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- W2000661497 abstract "The vibrational dynamics of the first four antisymmetric stretch vibrational levels of azide in an ionic glass have been measured and correlated using a heterodyned fifth-order two-dimensional infrared pulse sequence. By rephasing a two-quantum coherence, a process not possible with third-order spectroscopy, solvent effects on the frequencies and anharmonicities of the potential energy surface are measured. Fifth-order pulse sequences are another step towards precisely controlling vibrational coherence in analogy to the manipulation of spins in NMR but with ultrafast time resolution." @default.
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- W2000661497 date "2005-02-16" @default.
- W2000661497 modified "2023-10-02" @default.
- W2000661497 title "Vibrational Dynamics of Ions in Glass from Fifth-Order Two-Dimensional Infrared Spectroscopy" @default.
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- W2000661497 doi "https://doi.org/10.1103/physrevlett.94.067402" @default.
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