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• W2000684609 abstract "The reduction of CO2 and H+ by Ni(cyclam)+ in aqueous solution was found to proceed by the reduction of Ni(cyclam)(CO2)+ or Ni(cyclam)(H)2+ by Ni(cyclam)+. At ambient temperature the rate constants for the bimolecular reactions are 1.6 × 108 and 7.2 × 107 M-1 s-1, respectively. Continuous γ-radiolysis studies have demonstrated nearly quantitative formation of CO from two Ni(cyclam)+ at pH 5.2 under 1 atm of CO2 and in the presence of formate. Under the same conditions, but at low CO2 concentration, the reduction of protons was found to compete with CO2 reduction." @default.
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• W2000684609 date "1999-03-16" @default.
• W2000684609 modified "2023-09-27" @default.
• W2000684609 title "Mechanism of CO₂ and H⁺ Reduction by Ni(cyclam)⁺ in Aqueous Solution. A Pulse and Continuous Radiolysis Study" @default.
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• W2000684609 doi "https://doi.org/10.1021/ic980902p" @default.
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