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- W2000691773 abstract "Abstract The kinetics of hydrogen reduction of UO 3 and U 3 O 8 derived from the calcination of ammonium diuranate were studied by thermo-gravimetric analysis between 500 and 650°C at atmospheric pressure over a range of hydrogen concentrations. Calcination of ammonium diuranate produced UO 3 below about 600°C and U 3 O 8 above 600°C. The reduction of UO 3 took place in two steps: UO 3 to U 3 O 8 and U 3 O 8 to UO 2 . The order of reaction with respect to unconverted solid was zero for the UO 3 to U 3 O 8 step and varied from 0·65 to zero for the U 3 O 8 to UO 2 step depending on hydrogen concentration and temperature. For both reactions, the order with respect to hydrogen concentration was 0·9. The activation energies were 44·0 kJ mol −1 for the UO 3 to U 3 O 8 reaction and 88·5 kJ mol −1 for the U 3 O 8 to UO 2 reaction." @default.
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- W2000691773 date "1974-01-01" @default.
- W2000691773 modified "2023-09-26" @default.
- W2000691773 title "The kinetics of hydrogen reduction of UO3 and U3O8 derived from ammonium diuranate" @default.
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- W2000691773 doi "https://doi.org/10.1016/0022-1902(74)80663-9" @default.
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