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• W2000704296 abstract "Observations of the NO 2 column and its diurnal variation provide an important test of aspects of stratospheric chemistry. Measurements of NO 2 from two sites in the Antarctic are compared with model calculations that include a detailed treatment of diurnal NO x : chemistry for fall, winter, and spring. Observed slant column amounts in spring provide strong evidence for important heterogeneous effects, probably through polar stratospheric cloud chemistry. It is shown that the slow growth of NO 2 column observed during September is consitent with release of NO 2 from N 2 O 5 formed above the altitudes where polar stratospheric clouds occur. The observed early fall column amounts are in good agreement with model calculations, and the sharp onset of diurnal variation in column NO 2 obtained near day 57 is well stimulated. Following this period, gas‐phase model calculations suggest that N 2 O 5 will rapidly accumulate during the Antarctic fall as nights become longer. It is suggested that the high latitude fall period during which N 2 O 5 grows rapidly represents an optimum time to search for evidence of possible heterogeneous chemistry on background aerosols." @default.
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• W2000704296 date "1992-05-30" @default.
• W2000704296 modified "2023-09-26" @default.
• W2000704296 title "Seasonal variations in Antarctic NO_<i>x</i>chemistry" @default.
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• W2000704296 doi "https://doi.org/10.1029/91jd01707" @default.
• W2000704296 hasPublicationYear "1992" @default.
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