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- W2000716403 abstract "A nonlocal and non-Gaussian expression for the effective Hamiltonian of a fluctuating liquid-vapor interface is derived from the density functional theory for inhomogeneous simple fluids. After applying a gradient expansion one obtains as the leading term the standard capillary-wave Hamiltonian. The next to leading terms are proportional to the Gaussian curvature and to the mean curvature squared. Microscopic expressions for the coefficients in this expansion are derived. The breakdown of the gradient expansion for long-range interparticle forces is pointed out; this break-down is also reflected in the nonanalytical behavior of the (microscopically derived) wave-vector-dependent surface tension. The connection between recent scattering experiments and the derived Hamiltonian is discussed." @default.
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- W2000716403 date "1994-03-01" @default.
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- W2000716403 title "Structure of the effective hamiltonian for liquid-vapor interfaces" @default.
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- W2000716403 doi "https://doi.org/10.1002/bbpc.19940980313" @default.
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