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• W2000748913 abstract "We have measured the temperature dependence of reflectivity spectra of a single crystal of (C2H5)2(CH3)2Sb[Pd(dmit)2]2 (dmit = 1,3-dithiol-2-thione-4,5-dithiolate), to elucidate the origin of its phase transition at 70 K. A remarkable splitting has been found for the bonding–antibonding excitation of the dimer, [Pd(dmit)2]2, in the low-temperature phase. This manifests that the phase transition is due to the charge separation, 2 dimer− → dimer0 + dimer2−. This result, supporting our quantum chemical model for a strongly dimerized two-orbital system, gives a clue to incorporate a new spin–charge–orbital interplay in a molecular assembly." @default.
• W2000748913 created "2016-06-24" @default.
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• W2000748913 date "2005-08-01" @default.
• W2000748913 modified "2023-10-16" @default.
• W2000748913 title "Spectroscopic evidence for the low-temperature charge-separated state of [Pd(dmit)2] salts" @default.
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• W2000748913 doi "https://doi.org/10.1016/j.cplett.2005.06.026" @default.
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