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- W2000773055 abstract "Abstract The investigation of Ru/Mn/Ce/Al 2 O 3 catalyst on the ceria loading, calcination temperature and catalyst dosage had significantly affected the catalytic performance. The optimum conditions were achieved over 10 g of Ru/Mn/Ce/Al 2 O 3 catalysts calcined at 1000 °C with 65 wt% of Ce loading which gave 97.73% CO 2 conversion and 91.31% of methane formation at reaction temperature of 200 °C. The physicochemical properties investigated by XRD diffractogram showed that the catalyst still having polycrystalline structure with the mixture of Mn 4+ and Mn 3+ although had being calcined at high temperature of 1000 °C. Meanwhile, FESEM analysis indicated a morphology which looks like staghorn coral morphology with the smallest particle size of 86 nm and the highest BET surface area of 47.65 m 2 /g. The impact of these three critical parameters was investigated via Box–Behnken experimental design and their optimum values obtained over 10 g of Ru/Mn/Ce/Al 2 O 3 catalyst were calcined at 1025 °C with Ce loading of 65 wt%. The predicted value given was 98.95% of CO 2 conversion which was closely agreed with our experimental result (98.25%) over similar conditions." @default.
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- W2000773055 date "2014-09-01" @default.
- W2000773055 modified "2023-09-24" @default.
- W2000773055 title "Investigation of Ru/Mn/Ce/Al2O3 catalyst for carbon dioxide methanation: Catalytic optimization, physicochemical studies and RSM" @default.
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- W2000773055 doi "https://doi.org/10.1016/j.jtice.2014.07.009" @default.
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