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- W2000799124 abstract "The variation of the collisionless absorption spectral shapes for vibrationally excited SF<sub>6</sub> and C<sub>2</sub>F<sub>5</sub>C1 as a function of the picosecond probe pulse duration was determined using a two-IR frequency pump-probe scheme. The experiments revealed a spectral narrowing with decreasing pulse duration, similar to a recent observation in C<sub>3</sub>F<sub>7</sub>I with a single laser pulse. The observed experimental results are shown to be consistent with a dynamic multi-tier classification of energy levels in the QC of polyatomic molecules. Specifically, the time constants for such a coupling are evaluated to be >20 ps for all the molecules studied." @default.
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- W2000799124 date "1987-01-01" @default.
- W2000799124 modified "2023-09-23" @default.
- W2000799124 title "Picosecond Dynamical Temporal Evolution Of Molecular Ir Absorption Spectra" @default.
- W2000799124 doi "https://doi.org/10.1117/12.966900" @default.
- W2000799124 hasPublicationYear "1987" @default.
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