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• W2000833189 abstract "Abstract We present the first direct kinetic study of the reaction Pb + N2O → PbO + N2, by time-resolved atomic resonance absorption spectroscopy. Pb(63P0) was generated by the low energy pulsed irradiation of PbBr2 vapour in equilibrium with its solid at elevated temperatures and monitored in the “single-shot mode” by attenuation of the resonance transition at λ = 283.3 nm (Pb(73P°1) « Pb(63P0)). Absolute second-order rate constants for the process (kN2O were measured across the temperature range 648 – 783 K yielding the Arrhenius form (error 1σ in Eact). There is an uncertainty of a factor of about 2 in the Arrhenius A parameter. This measurement is compared with analogous data for other group IV atoms in their 3P ground states, including Arrhenius parameters for the processes Sn(53P0) + N2O and Ge(43PJ) + N2O derived from time-resolved resonance absorption spectroscopy and high temperature fast flow reactor measurements. Single temperature rate data for C(23PJ) and Si(33PJ) with N2O are also considered. Finally, the feasibility of observing chemiluminescence via the a → X and b → X systems of PbO from Pb + N2O is discussed." @default.
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• W2000833189 date "1986-12-01" @default.
• W2000833189 modified "2023-09-25" @default.
• W2000833189 title "The reaction of Pb(63P0) with N2O at elevated temperatures studied by time-resolved atomic resonance absorption spectroscopy" @default.
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• W2000833189 doi "https://doi.org/10.1016/0047-2670(86)87057-5" @default.
• W2000833189 hasPublicationYear "1986" @default.
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