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• W2000840417 abstract "High-resolution photoemission spectroscopy and ab initio calculations have been employed to analyze the onset and progression of $dmathrm{text{ensuremath{-}}}sp$ hybridization in Fe impurities deposited on alkali metal films. The interplay between delocalization, mediated by the free-electron environment, and Coulomb interaction among $d$ electrons gives rise to complex electronic configurations. The multiplet structure of a single Fe atom evolves and gradually dissolves into a quasiparticle peak near the Fermi level with increasing host electron density. The effective multiorbital impurity problem within the exact diagonalization scheme describes the whole range of hybridizations." @default.
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• W2000840417 date "2010-03-15" @default.
• W2000840417 modified "2023-10-18" @default.
• W2000840417 title "Correlated Electrons Step by Step: Itinerant-to-Localized Transition of Fe Impurities in Free-Electron Metal Hosts" @default.
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• W2000840417 doi "https://doi.org/10.1103/physrevlett.104.117601" @default.
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