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• W2000846148 abstract "We examine the utility of photoelectron spectroscopy (PES) as a structural probe of Sin− in the n=20–26 size range by determining isomers and associated photoelectron spectra from first principles calculations. Across the entire size range, we consistently obtain a good agreement between the theory and experiment [Hoffmann et al., Eur. Phys. J. D 16, 9 (2001)]. We find that PES can almost invariably distinguish between structurally distinct isomers at a given cluster size, but that structurally similar isomers usually cannot be reliably distinguished by PES. For many, but not all, sizes the isomer giving the best match to experiment is the lowest-energy one found theoretically. Thus, combining theory with PES experiments emerges as a useful source of structural information even for intermediate size clusters." @default.
• W2000846148 created "2016-06-24" @default.
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• W2000846148 date "2005-11-22" @default.
• W2000846148 modified "2023-10-18" @default.
• W2000846148 title "Photoelectron spectroscopy as a structural probe of intermediate size clusters" @default.
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• W2000846148 doi "https://doi.org/10.1063/1.2116907" @default.
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