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• W2000871529 abstract "A new theoretical approach is presented for vapor-phase nucleation. In contrast to previous molecular approaches to nucleation that focus on evaluating equilibrium distributions of clusters, we evaluate rate constants for cluster evaporation and condensation that are the elementary kinetic steps in the nucleation mechanism. The use of variational transition state theory to estimate the rate constants provides a consistent procedure for defining a unique value for the constraining volume of the physically consistent cluster. The theory is applied to evaporation of small water clusters." @default.
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• W2000871529 date "1999-04-26" @default.
• W2000871529 modified "2023-10-12" @default.
• W2000871529 title "Dynamical Nucleation Theory: A New Molecular Approach to Vapor-Liquid Nucleation" @default.
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• W2000871529 doi "https://doi.org/10.1103/physrevlett.82.3484" @default.
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