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• W2000885277 abstract "We studied the reaction kinetics of sulfur oxidation on the Pd(100) surface by in situ high resolution x-ray photoelectron spectroscopy and ab initio density functional calculations. Isothermal oxidation experiments were performed between 400 and 500 K for small amounts (∼0.02 ML) of preadsorbed sulfur, with oxygen in large excess. The main stable reaction intermediate found on the surface is SO4, with SO2 and SO3 being only present in minor amounts. Density-functional calculations depict a reaction energy profile, which explains the sequential formation of SO2, SO3, and eventually SO4, also highlighting that the in-plane formation of SO from S and O adatoms is the rate limiting step. From the experiments we determined the activation energy of the rate limiting step to be 85 ± 6 kJ mol−1 by Arrhenius analysis, matching the calculated endothermicity of the SO formation." @default.
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• W2000885277 date "2012-03-01" @default.
• W2000885277 modified "2023-10-18" @default.
• W2000885277 title "Kinetics of the sulfur oxidation on palladium: A combined <i>in situ</i> x-ray photoelectron spectroscopy and density-functional study" @default.
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• W2000885277 doi "https://doi.org/10.1063/1.3687676" @default.
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