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- W2000889622 abstract "The kinetics of crystalline ice nucleation and growth in nonporous, molecular beam deposited amorphous solid water (ASW) films are investigated at temperatures near 140 K. We implement an experimental methodology and corresponding model of crystallization kinetics to decouple growth from nucleation and quantify the temperature dependence and absolute rates of both processes. Nucleation rates are found to increase from approximately 3x10(13) m(-3) s(-1) at 134 K to approximately 2x10(17) m(-3) s(-1) at 142 K, corresponding to an Arrhenius activation energy of 168 kJ/mol. Over the same temperature range, the growth velocity increases from approximately 0.4 to approximately 4 A s(-1), also exhibiting Arrhenius behavior with an activation energy of 47 kJ/mol. These nucleation rates are up to ten orders of magnitude larger than in liquid water near 235 K, while growth velocities are approximately 10(9) times smaller. Crystalline ice nucleation kinetics determined in this study differ significantly from those reported previously for porous, background vapor deposited ASW, suggesting the nucleation mechanism is dependent upon film morphology." @default.
- W2000889622 created "2016-06-24" @default.
- W2000889622 creator A5036746714 @default.
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- W2000889622 date "2004-09-22" @default.
- W2000889622 modified "2023-09-23" @default.
- W2000889622 title "The nucleation rate of crystalline ice in amorphous solid water" @default.
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- W2000889622 doi "https://doi.org/10.1063/1.1779171" @default.
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