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• W2000893465 abstract "The state-resolved reactivity of ${mathrm{CH}}_{4}$ in its totally symmetric C-H stretch vibration (${ensuremath{nu}}_{1}$) has been measured on a Ni(100) surface. Methane molecules were accelerated to kinetic energies of 49 and $63.5text{ }text{ }mathrm{kJ}/mathrm{mol}$ in a molecular beam and vibrationally excited to ${ensuremath{nu}}_{1}$ by stimulated Raman pumping before surface impact at normal incidence. The reactivity of the symmetric-stretch excited ${mathrm{CH}}_{4}$ is about an order of magnitude higher than that of methane excited to the antisymmetric stretch (${ensuremath{nu}}_{3}$) reported by Juurlink et al. [Phys. Rev. Lett. 83, 868 (1999)] and is similar to that we have previously observed for the excitation of the first overtone ($2{ensuremath{nu}}_{3}$). The difference between the state-resolved reactivity for ${ensuremath{nu}}_{1}$ and ${ensuremath{nu}}_{3}$ is consistent with predictions of a vibrationally adiabatic model of the methane reaction dynamics and indicates that statistical models cannot correctly describe the chemisorption of ${mathrm{CH}}_{4}$ on nickel." @default.
• W2000893465 created "2016-06-24" @default.
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• W2000893465 date "2005-06-22" @default.
• W2000893465 modified "2023-10-18" @default.
• W2000893465 title "State-Resolved Gas-Surface Reactivity of Methane in the Symmetric C-H Stretch Vibration on Ni(100)" @default.
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• W2000893465 doi "https://doi.org/10.1103/physrevlett.94.246104" @default.
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