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• W2000914174 abstract "The interaction of He(23S) with CS2 produces relatively strong emission from the CS+(A2II−X2∑+) and CS(A1II−X1∑+) systems; weaker emission is observed from CS2+(A2IIu−X2IIg), CS2+(B2∑u+−X2IIg), CS(a3II−X1∑+), some unassigned transitions, and atomic emission (mainly from S*) in the vacuum ultraviolet. Several new CS+(A−X) emission bands were observed and these yield improved spectroscopic constants for both the CS+(X) and CS+(A) states. Available data for ΔHfoQ(CS) are critically assessed, and estimates of ΔHfoQ(CS+)=326.4±0.7 and D00(CS+)=147.8±0.9 kcal mole−1 are obtained. The experimentally observed band intensities were combined with Franck-Condon factors calculated from a Morse potential for CS+(X) and an RKR potential for CS+(A) to obtain vibrational populations, and to compare calculated and experimental radiative branching ratios. The band intensities from the CS(A1II, v′=0–4) levels were combined with calculated RKR Franck-Condon factors to analyze the dependence of the electronic transition moment on r-centroid. The other emission systems observed from the He(23S)+CS2 reaction also are summarized, and some aspects of the quenching mechanism are discussed and compared to the photoionization of CS2." @default.
• W2000914174 created "2016-06-24" @default.
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• W2000914174 date "1976-11-01" @default.
• W2000914174 modified "2023-09-23" @default.
• W2000914174 title "Intensity and wavelength measurements for the CS+ (A2II−X2∑+) and CS(A1II−X1∑+) band systems excited by the reaction of metastable He(23S) with CS2" @default.
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• W2000914174 doi "https://doi.org/10.1016/s0301-0104(76)80004-3" @default.
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