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- W2000932911 abstract "Reaction of carbon dioxide with butadiene catalyzed by palladium–phosphine complexes was studied. When the reaction was carried out in certain polar, aprotic solvents, such as dimethylformamide (DMF), 2-ethylidene-5-hepten-4-olide was formed in about 5% yield by the incorporation of CO2 together with the formation of butadiene linear dimers. The main dimer was 1,3,7-octatriene. The ditertiary phosphines, R2PCH2CH2CH2PR2 where R is methyl or phenyl, were found to be suitable as the ligand for the olide synthesis. A possible mechanism involving the intermediate of π-allyl, σ-allyl form from two moles of butadiene and the palladium complex is proposed." @default.
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- W2000932911 date "1978-08-01" @default.
- W2000932911 modified "2023-10-14" @default.
- W2000932911 title "Incorporation of CO<sub>2</sub>in Butadiene Dimerization Catalyzed by Palladium Complexes. Formation of 2-Ethylidene-5-hepten-4-olide" @default.
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- W2000932911 doi "https://doi.org/10.1246/bcsj.51.2375" @default.
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