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• W2000933548 abstract "Abstract Transition-metal-catalyzed C–H functionalizations have emerged as complementary and powerful tools to access molecular complexity from widely available starting materials. Herein, we present a strategy for asymmetric intramolecular Pd(0)-catalyzed C–H functionalizations. The outlined reactivity is based on the cooperative effect between a chiral phosphorous ligand and a carboxylate base acting as a relay of chirality during the enantio-discriminating concerted metalation deprotonation step. This approach allows the enantioselective construction of a range of important semi-saturated chiral nitrogen-containing heterocycles such as indolines, tetrahydroquinolines, and dibenzazepinones." @default.
• W2000933548 created "2016-06-24" @default.
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• W2000933548 date "2014-03-04" @default.
• W2000933548 modified "2023-10-02" @default.
• W2000933548 title "Enantioselective palladium(0)-catalyzed C–H arylation strategy for chiral heterocycles" @default.
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• W2000933548 doi "https://doi.org/10.1515/pac-2014-5029" @default.
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