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• W2000936423 abstract "In lithium ion batteries, decomposition of the electrolyte and its associated passivation of the electrode surface occurs at low potentials, resulting in an electronically insulating, but Li-ion conducting, solid electrolyte interphase (SEI). The products of the SEI and their chemical constituents/properties play an important role in the long-term stability and performance of the battery. Reactivity and the sub-keV core binding energies of lithium, carbon, oxygen, and fluorine species in the SEI present technical challenges in the spectroscopy of these compounds. Using an alternative approach, nonresonant inelastic x-ray scattering, we examine the near-edge spectra of bulk specimens of common SEI compounds, including LiF, Li2CO3, LiOH, LiOH·H2O, and Li2O. By working at hard x-ray energies, we also experimentally differentiate the s- and p-symmetry components of lithium's unoccupied states using the evolution of its K edge with momentum transfer. We find good agreement with theoretical spectra calculated using a Bethe-Salpeter approach in all cases. These results provide an analytical and diagnostic foundation for better understanding of the makeup of SEIs and the mechanism of their formation." @default.
• W2000936423 created "2016-06-24" @default.
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• W2000936423 date "2011-12-13" @default.
• W2000936423 modified "2023-10-16" @default.
• W2000936423 title "Electronic structure of lithium battery interphase compounds: Comparison between inelastic x-ray scattering measurements and theory" @default.
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• W2000936423 doi "https://doi.org/10.1063/1.3664620" @default.
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