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- W2000950421 abstract "The rate constant, macroscopic branching ratio and vibrational distribution for the reaction O(1D) + H2S→OH + SH were measured. Temporal dependencies of the OH radical concentration in different ro-vibronic states were monitored by the LIF technique after laser flash photolysis of ozone which generated O(1D) atoms. The total rate constant was found to be (2.2±0.5 ) × 10−10 cm−3 molecule−1 s−1. The relative fraction of channel producing OH and SH radicals is 0.26 ± 0.04. The vibrational distribution of OH radicals P(ν=0): P(ν= 1) : P (ν=2) : P(ν=3) : P(ν=4) : P(ν=5) = 0.19:0.21:0.26:0.2:0.11:0.03 is similar to that for the reaction of O (1D) atoms with H2, CH4 and NH3 which indicates the similar dynamics of these reactions." @default.
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- W2000950421 date "1993-09-01" @default.
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- W2000950421 title "Formation of vibrationally excited OH radicals in the O (1D) + H2S reaction" @default.
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- W2000950421 doi "https://doi.org/10.1016/0009-2614(93)85492-7" @default.
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