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- W2001099511 abstract "Abstract Proton magnetic relaxation rates in the system N(CH) 3 ) 4 Br/NiBr 2 /D 2 O, N(CH 3 ) 4 Br/MnBr 2 / D 2 O, Ni(00CCH 3 ) 2 /D 2 O and Mn(00CCH 3 ) 2 /D 2 O have been measured as a function of the solute concentration in the range 0.002 < c* ⪍ 1 m. Division by the concentration c* and by a quantity characterizing the ionic motion yields the association parameter (4-parameter). A decreases and increases with decreasing concentration for the systems involving cation-cation and cation-anion interaction, respectively. The relaxation rates of 35 C1 - , 133 Cs + , and 25 Mg ++ in diamagnetic aqueous solutions have also been measured down to high dilution. Here as well in most cases we have found an increase of the A-parameter with decreasing salt concentration, indicating ion-ion association at high dilution. A comparison with the results of the Debye-Hückel theory is given; there is qualitative agreement. Our experimental results for 35 C1 - generally do not support theoretical considerations in the literature, where a Cl - -Cl - association was postulated" @default.
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- W2001099511 date "1995-05-01" @default.
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- W2001099511 title "Ion-Ion De-Association and Association of Strong Electrolytes at High Dilution from Nuclear Magnetic Relaxation Measurements" @default.
- W2001099511 doi "https://doi.org/10.1515/zna-1995-4-523" @default.
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