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• W2001330962 abstract "The reactions of Pb atoms with molecular reagents F2 and Cl2 have been studied in a molecular beam apparatus by laser fluorescence detection of PbF and PbCl products. The experiments were performed in a beam-gas configuration under single-collision conditions. The PbCl product from Pb+Cl2 was observed in the vibrational levels v≤17 of the ground X1 electronic state. The PbCl product vibrational state distribution was derived; the average vibrational excitation was found to be 21% of the total available energy. For Pb+F2, PbF(X1) product was detected in only the v=0 and 1 vibrational levels, and the rovibrational state distribution could be characterized by a 300 K Boltzmann distribution. By modulating the Pb beam, it was concluded that this observed product was an artifact and did not arise from bimolecular gas-phase collisions. The radiative lifetimes of the PbF(A,B) and PbCl(A) states were also measured and were found to equal 4.9±0.3 μs, &lt;10 ns, and 1.14±0.06 μs, respectively, averaged over the observed vibrational levels." @default.
• W2001330962 created "2016-06-24" @default.
• W2001330962 creator A5048379858 @default.
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• W2001330962 date "1992-01-15" @default.
• W2001330962 modified "2023-09-23" @default.
• W2001330962 title "Laser fluorescence study of the Pb+F2, Cl2 reactions: Internal state distribution of the PbCl product and radiative lifetimes of PbF(<i>A</i>,<i>B</i>) and PbCl(<i>A</i>)" @default.
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• W2001330962 doi "https://doi.org/10.1063/1.462189" @default.
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