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- W2001349303 abstract "Spent fuel dissolution rates have been measured using a flowthrough system where the uranium concentrations remained well below solubility limits, thus allowing unambiguous reaction rates to be determined. The study was based on a statistically designed test matrix that covered four water chemistry variables: temperature (25 to 75°C), pH (8 to 10), carbonate/bicarbonate concentration (2 × 10−4M to 2 × 10−2M), and oxygen fugacity (O2 partial pressure 0.002 to 0.2 atm). Results obtained to date and reported here encompass the first three, all at 0.2 atm O2 partial pressure. The dissolution rate was found to be moderately dependent on temperature but only weakly dependent on pH and carbonate/bicarbonate concentration." @default.
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- W2001349303 date "1992-08-01" @default.
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- W2001349303 title "Parametric study of LWR spent fuel dissolution kinetics" @default.
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- W2001349303 doi "https://doi.org/10.1016/0022-3115(92)90074-u" @default.
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