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• W2001458251 abstract "C2-symmetric bis(oxazoline)−Cu(II) complexes 1 catalyze the Mukaiyama Michael reaction of alkylidene malonates and enolsilanes. The use of hexafluoro-2-propanol is essential to induce catalyst turnover. High enantioselectivities are exhibited by bulky alkylidene malonate β-substituents using catalyst 1a. The glutarate ester products are readily decarboxylated to provide chiral 1,5-dicarbonyl synthons. Crystallographic characterization of substrate−catalyst complexes provides insight into the binding event with these catalysts and affords a rationale for the observed facial selectivities." @default.
• W2001458251 created "2016-06-24" @default.
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• W2001458251 creator A5074994681 @default.
• W2001458251 date "2000-09-01" @default.
• W2001458251 modified "2023-10-11" @default.
• W2001458251 title "Enantioselective Lewis Acid Catalyzed Michael Reactions of Alkylidene Malonates. Catalysis by <i>C</i>₂-Symmetric Bis(oxazoline) Copper(II) Complexes in the Synthesis of Chiral, Differentiated Glutarate Esters" @default.
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• W2001458251 doi "https://doi.org/10.1021/ja002246+" @default.
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