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• W2001852263 abstract "Abstract The glass transition temperature of polymers and polymer solutions was approached through a combination of the group‐contribution, lattice‐fluid equation of state and the Gibbs–DiMarzio criterion. The model assumes zero entropy at the glass transition temperature and treats molecules as semiflexible chains. This stiffness is associated with a flex energy obtained from the glass transition temperature at atmospheric pressure. Whereas the application of the model is straightforward for homopolymers and polymer solutions, a new formalism using the dyad concept was developed for copolymers. It takes into account the copolymer composition as well as the sequencing of the monomers. The results obtained are consistent with experimental data. For polymer solutions, the model predictions are semiquantitative depending on the system. The interaction parameter required for binary systems was found to have little effect on the glass transition temperature predictions. © 2003 Wiley Periodicals, Inc. J Appl Polym Sci 89: 697–705, 2003" @default.
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• W2001852263 date "2003-05-02" @default.
• W2001852263 modified "2023-10-17" @default.
• W2001852263 title "A lattice-fluid, group-contribution treatment of the glass transition of homopolymers, copolymers, and polymer solutions" @default.
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• W2001852263 doi "https://doi.org/10.1002/app.12181" @default.
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