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- W2001911388 abstract "Various isotopologues of nature's simplest molecule, namely H2+, HD+, and D2+, have been isolated in neon matrices at 2 K for the first time and studied by electron spin resonance (ESR). Over many years, hundreds of matrix isolation experiments employing a variety of deposition conditions and ion generation methods have been tried to trap the H2+ cation radical in our laboratory. The molecule has been well characterized in the gas phase and by theoretical methods. The observed magnetic parameters for H2+ in neon at 2 K are: g∥ ≈ g⊥ = 2.0022(1); Aiso(H) = 881(7) MHz; and Adip(H) = 33(3) MHz. Reasonable agreement with gas phase values of the isotropic hyperfine interaction (Aiso) is observed; however, the neon matrix dipolar hyperfine interaction (Adip) is noticeably below the gas phase value. The smaller matrix value of Adip is attributable to motional averaging of the H2+ radical in the neon matrix trapping site–an occurrence that would prevent the full extent of the hyperfine anisotropy from being measured for a powder pattern type ESR sample." @default.
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- W2001911388 date "2012-11-28" @default.
- W2001911388 modified "2023-10-18" @default.
- W2001911388 title "Electron spin resonance investigation of H2+, HD+, and D2+ isolated in neon matrices at 2 K" @default.
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- W2001911388 doi "https://doi.org/10.1063/1.4767932" @default.
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