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• W2001958028 abstract "This study reports the interaction of acetaldehyde with well-ordered CeOX(111) thin film surfaces. The fully oxidized CeO2(111) surface shows a weak interaction with acetaldehyde with the sole desorption product (TPD) being the parent molecule at 210 K. The chemisorbed molecule binds to the surface as the η1-acetaldehyde species rather than through a bridge-bonded dioxy configuration. Acetaldehyde chemisorbs strongly on reduced CeO2−X(111) with nonrecombinative and recombinative acetaldehyde desorbing at 405 and 550−600 K, respectively. Deoxygenation and dehydration also occur, producing ethylene and acetylene at 580 and 620 K, respectively. Acetaldehyde initially adsorbs in the η1 configuration and then converts to a carbanion species with both C═C and C═O bond character above 300 K." @default.
• W2001958028 created "2016-06-24" @default.
• W2001958028 creator A5064484034 @default.
• W2001958028 creator A5086393561 @default.
• W2001958028 date "2011-02-07" @default.
• W2001958028 modified "2023-10-18" @default.
• W2001958028 title "Adsorption and Reaction of Acetaldehyde over CeO_<i>X</i>(111) Thin Films" @default.
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• W2001958028 doi "https://doi.org/10.1021/jp110429s" @default.
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