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- W2002008108 abstract "Electron-stimulated oxidation of CO in layered H2O/CO/H2O ices was investigated with infrared reflection–absorption spectroscopy (IRAS) as a function of the distance of the CO layer from the water/vacuum interface. The results show that while both oxidation and reduction reactions occur within the irradiated water films, there are distinct regions where either oxidation or reduction reactions are dominant. At depths less than ∼15 ML from the vacuum interface, CO oxidation to CO2 dominates over the sequential hydrogenation of CO to methanol (CH3OH), consistent with previous observations. At its highest yield, CO2 accounts for ∼45% of all the reacted CO. Another oxidation product is identified as the formate anion (HCO2–). In contrast, for CO buried more than ∼35 ML below the water/vacuum interface, the CO-to-methanol conversion efficiency is close to 100%. Production of CO2 and formate is not observed for the more deeply buried CO layers, where hydrogenation dominates. Experiments with CO dosed on preirrad..." @default.
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- W2002008108 date "2014-11-12" @default.
- W2002008108 modified "2023-09-24" @default.
- W2002008108 title "Distance-Dependent Radiation Chemistry: Oxidation versus Hydrogenation of CO in Electron-Irradiated H<sub>2</sub>O/CO/H<sub>2</sub>O Ices" @default.
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- W2002008108 doi "https://doi.org/10.1021/jp509785d" @default.
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