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- W2002089360 abstract "The structure of the unstable $c(2ifmmodetimeselsetexttimesfi{}2)$ Mn surface alloy that is formed on Ag(001) upon deposition of an Mn monolayer at room temperature is determined by low-energy electron diffraction (LEED). The optimized structure model is basically a two-monolayer-thick ${mathrm{Mn}}_{x}{mathrm{Ag}}_{100ensuremath{-}x}$ alloy that is ordered in a checkerboard arrangement in the first layer and random in the second layer, with substantial deviations from ideal order and stoichiometry $x=50.$ The surface alloy essentially prolongs the face-centered-cubic Ag lattice, with interlayer distances ${d}_{12}=1.985ifmmodepmelsetextpmfi{}0.010AA{}$ and ${d}_{23}=2.030ifmmodepmelsetextpmfi{}0.008AA{}$ only slightly reduced with respect to Ag bulk, and a buckling of 0.07 AA{} (Mn displaced outwards) in the top layer. The present work clearly confirms the unusually large atomic volume of Mn in this environment as found in previous surface-extended x-ray absorption fine structure work [P. Schieffer, M.-H. Tuilier, M.-C. Hanf, C. Krembel, G. Gewinner, D. Chandesris, and H. Magnan, Phys. Rev. B 57, 15 507 (1998)] and disproves the geometry inferred from an earlier LEED study [Wondong Kim, Wookje Kim, S.-J. Oh, J. Seo, J.-S. Kim, H.-G. Min, and S.-C. Hon, Phys. Rev. B 57, 8823 (1998)]." @default.
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- W2002089360 date "2002-06-13" @default.
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- W2002089360 title "Atomic structure of the Ag(001)c(2×2) Mn surface alloy" @default.
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- W2002089360 doi "https://doi.org/10.1103/physrevb.65.235427" @default.
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