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- W2002124001 abstract "We use DFT to investigate an atomistic mechanism for the ALD of hafnium nitride films grown using Hf[N(CH3)2]4 and NH3. We find a ligand-exchange mechanism similar to those thought to occur in the ALD of HfO2 using the same Hf source and H2O. Although the Hf[N(CH3)2]4 half-reaction at NH* sites has a barrier similar to that of reaction with OH* sites, the barrier for the NH3 half-reaction on the Hf[N(CH3)2]x∗ terminated surface is significantly larger than for reaction between H2O and Hf[N(CH3)2]x∗. Thus, the NH3 half-cycle will be prone to oxygen incorporation into Hf–nitride from residual H2O." @default.
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- W2002124001 date "2005-05-01" @default.
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- W2002124001 title "Atomic layer deposition of hafnium nitrides using ammonia and alkylamide precursors" @default.
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- W2002124001 doi "https://doi.org/10.1016/j.cplett.2005.03.084" @default.
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