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• W2002165683 abstract "Abstract The heat capacity of the mixed-valence complex 1′,1′″-diiodobiferrocenium triiodide, [(C 5 H 4 IFe) 2 (C 10 H 8 )] + I − 3 , has been measured by adiabatic calorimetry between 80 mK and 25 K. A Schottky anomaly centered around 0.6 K was found and interpreted in terms of a tunnel splitting of the vibronic ground state of the cation, which leads to a molecular quantum paraelectric (MQP). The splitting was determined to be ≈ 1 cm −1 which corresponds to an intermolecular electron transfer rate of ≈ 0.7 × 10 9 s −1 . The mean field theory by Kambara and Sasaki has been applied to determine the phase diagram. The MQP state is stable unless the cation—anion interaction exceeds ≈ 12.3 cm −1 . The possibility of a phase transition in the MQP under some external fields has been discussed." @default.
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• W2002165683 date "1992-08-01" @default.
• W2002165683 modified "2023-09-27" @default.
• W2002165683 title "Heat capacity of mixed-valence 1′,1′″-diiodobiferrocenium triiodide in the 0.080–25 K range: direct observation of tunnel splitting" @default.
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• W2002165683 doi "https://doi.org/10.1016/0009-2614(92)85725-p" @default.
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