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• W2002204044 abstract "The vibrational relaxation of a diatomic molecule adsorbed on a surface is studied using a quantum mechanical model which explicitly takes into account the coupling to the anharmonic adbond vibration. The intramolecular vibrational frequency is assumed to be much higher than the phonon frequency, and it is described as a two‐level system. The molecule–surface adbond is taken to be a Morse oscillator which is anharmonically coupled to the fluctuating bath. The bath is a Debye distribution of harmonic oscillators. A closed expression is derived for the relaxation rate which is shown to include contributions from different channels. The most important channel for the energy flow consists of near (nonlinear) resonance energy transfer from the molecular vibrational mode to the adbond, accompanied by low‐order (one or two) emission/absorption of phonons. The theory is applied to the relaxation of OH on silica and can reproduce quantitatively the measured relaxation rate and its temperature dependency." @default.
• W2002204044 created "2016-06-24" @default.
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• W2002204044 date "1989-06-15" @default.
• W2002204044 modified "2023-09-27" @default.
• W2002204044 title "A quantum theoretic model of vibrational relaxation of a diatomic molecule adsorbed on a surface" @default.
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• W2002204044 doi "https://doi.org/10.1063/1.456187" @default.
• W2002204044 hasPublicationYear "1989" @default.
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