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- W2002244993 abstract "The gas phase exchange reaction with stoichiometry 13C 16O+12C 18O→13C 18O+12C 16O has been studied using a mercury photosensitization technique. The mechanism of the photosensitized exchange reaction is complex and almost certainly involves electronically excited CO(a 3Π). No evidence for a simple bimolecular exchange mechanism involving ground electronic state, vibrationally excited CO was found, although such a mechanism is not conclusively ruled out by the photosensitization experiments for vibrational levels higher than 9. Since such a mechanism has previously been proposed based on shock tube studies, a computer simulation of the shock tube exchange reaction was undertaken. One set of shock tube experiments can be reinterpreted quite well in terms of an atomic chain mechanism initiated by traces of O2 impurity. The mechanism of the second set remains a mystery." @default.
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- W2002244993 date "1984-06-15" @default.
- W2002244993 modified "2023-09-28" @default.
- W2002244993 title "On the mechanism of the CO self-exchange reaction" @default.
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- W2002244993 doi "https://doi.org/10.1063/1.446687" @default.
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