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- W2002602758 abstract "Composites comprising alkali metal alloys and alkali metal doped conductive polymers constitute a class of electrode materials useful in rechargeable cells. Composite electrodes made with poly(p-phenylene) (PPP) and polyacetylene (PA) exhibit high rechargeability for donor doping (cation insertion) in ether electrolytes such as NaPF6 in 1,2-dimethoxyethane (DME) and LiPF6 in 2-methyltetrahydrofuran (MTHF), plus rechargeability, at restricted potentials, in solvents such as sulfolane and benzonitrile. NaPb, LiPb, and LiAl alloys, formed as composites with PPP and PA, have been cycled exhaustively with excellent charge capacity retention. These composites form rechargeable cells with a variety of cation-inserting cathodes. In particular, balanced cells having NaPb/PPP anodes and NaCoO2 cathodes have been cycled 250 times with little capacity loss. The good performance of these composites is due, in part, to the basic fibrillar morphology of the polymer, which becomes evident during cycling. After several cycles, the composites possess the fibrillar structure of pure polymer electrodes, with crystalline alloy uniformly distributed on or in the fibrils in particles of less than 0.2 μm. This structure, particularly when the fibrils are swollen with electrolyte, facilitates rapid transport of ions and electronic charge throughout the electrode." @default.
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- W2002602758 date "1989-05-01" @default.
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- W2002602758 title "Alloy/conducting-polymer composite electrodes: electrolytes, cathodes, and morphology" @default.
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- W2002602758 doi "https://doi.org/10.1016/0378-7753(89)80018-7" @default.
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