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• W2002755553 abstract "X-Ray powder analysis shows that the Mn 2 Sb phase has a very narrow range of homogeneity below 700 °C. The composition of the phase is approximately Mn 2.10 Sb at 250 °C and includes the stoichiometric ratio Mn 2.00 Sb at 700 °C. Heat capacity measurements on samples with these two compositions have been carried out. Λ-Type maxima occasioned by the ferri- to paramagnetic transition in the samples are noted at 273 °C in Mn 2.00 Sb and at 279 °C in Mn 2.10 Sb. A further effect is observed for Mn 2.00 Sb in the range 250 to 450 °C, and attributed to the changing composition of the Mn 2 Sb phase. Values of heat capacities and enthalpy and entropy increments are tabulated for selected temperatures up to 1000 K for Mn 2.00 Sb and to 700 K for Mn 2.10 Sb. For Mn 2.00 Sb the enthalpy increment H o (1000 K) − H o (298 K) = 70 360 J mol −1 and the entropy increment S o (1000 K) − S o (298 K) = 120.1 J mol −1 K −1 . A tentative resolution of the cooperative magnetic component leads to ΔH m = 6860 J mol −1 and ΔS m = 16.4 J mol −1 K −1 . Further magnetic contributions of less cooperative nature are probably present, and more energy states available than the spin-only states of 2(1.77) and 4(3.55) 3d-electrons, respectively, for the two types of manganese atom." @default.
• W2002755553 created "2016-06-24" @default.
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• W2002755553 date "1969-03-01" @default.
• W2002755553 modified "2023-09-24" @default.
• W2002755553 title "The Mn2Sb phase composition and thermodynamic properties in the range 298 to 1000 K" @default.
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• W2002755553 doi "https://doi.org/10.1016/0021-9614(69)90054-8" @default.
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