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- W2002907925 abstract "The complete initial distribution of product vibrational and rotational state populations for the following energy transfer process has been determined for Boltzmann conditions at ∼550°K.: The initial population distribution of NO(A 2Σ+, v′=1) rotational levels is remarkably consistent with that predicted by the Cross–Gordon version of near-resonant dipole–dipole theory, except that a minor (∼7%) Boltzmann-like population must be included for satisfactory simulation of the sensitized NO γ (1,X) band spectra in the frequency regions dominated by transitions originating from lower rotational levels. The initial rotational level population distribution of NO (A 2Σ+, v′=0) is very similar to a Boltzmann population distribution at ∼1400°K. The rate of production of NO(A 2Σ+, v′=1) is ∼10 times that of NO(A 2Σ+, v′=0). Efficient ’’near-resonant’’ dipole–dipole interactions appear, therefore, to constitute the dominant mechanism for electronic energy transfer in this particular system. Production of NO(A 2Σ+, v′=0), and possibly the lower rotational levels of NO(A 2Σ+, v′=1), likely result from a minor competing mechanism. A Zn+NO− charge-transfer surface crossing is suggested as one possibility." @default.
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- W2002907925 date "1979-05-15" @default.
- W2002907925 modified "2023-09-27" @default.
- W2002907925 title "Near-resonant electronic energy transfer: Initial rotational state populations of NO(<i>A</i> 2Σ+, <i>v</i>′=0,1) produced by energy transfer from Zn(1<i>P</i>1)" @default.
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- W2002907925 doi "https://doi.org/10.1063/1.437264" @default.
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